Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties

M. J. Nystrom; B. W. Wessels; D. A. Neumayer; Tobin J Marks; W. P. Lin; G. K. Wong

Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties

M. J. Nystrom, B. W. Wessels, D. A. Neumayer, Tobin J Marks, W. P. Lin, G. K. Wong

Northwestern University

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

3 Citations (Scopus)

Abstract

Single phase, highly textured strontium barium niobate (SBN) thin films were deposited by low pressure metal-organic chemical vapor deposition on both crystalline and amorphous substrates. The metal precursors employed were niobium pentaethoxide as well as barium and strontium (hexafluoroacetylacetonate)₂·tetraglyme. SBN thin films with compositions across the entire solid solution range were deposited. The nonlinear optical properties of the SBN films were also measured. Nonlinear optical coefficients approaching bulk values were obtained for as-deposited oriented films. The room temperature, effective second-order nonlinear coefficient was 3.0 pm/V. Films with the highest degree of crystalline perfection had the largest effective nonlinear coefficient. The second harmonic intensity was strongly temperature dependent with a maximum at the ferroelectric transition.

Original language	English
Title of host publication	Materials Research Society Symposium - Proceedings
Publisher	Materials Research Society
Pages	167-172
Number of pages	6
Volume	361
Publication status	Published - 1995
Event	Proceedings of the 1994 MRS Fall Meeting - Boston, MA, USA Duration: Nov 29 1994 → Dec 2 1994

Other

Other	Proceedings of the 1994 MRS Fall Meeting
City	Boston, MA, USA
Period	11/29/94 → 12/2/94

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials

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Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties. / Nystrom, M. J.; Wessels, B. W.; Neumayer, D. A.; Marks, Tobin J; Lin, W. P.; Wong, G. K.

Materials Research Society Symposium - Proceedings. Vol. 361 Materials Research Society, 1995. p. 167-172.

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Nystrom, MJ, Wessels, BW, Neumayer, DA, Marks, TJ, Lin, WP & Wong, GK 1995, Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties. in Materials Research Society Symposium - Proceedings. vol. 361, Materials Research Society, pp. 167-172, Proceedings of the 1994 MRS Fall Meeting, Boston, MA, USA, 11/29/94.

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title = "Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties",

abstract = "Single phase, highly textured strontium barium niobate (SBN) thin films were deposited by low pressure metal-organic chemical vapor deposition on both crystalline and amorphous substrates. The metal precursors employed were niobium pentaethoxide as well as barium and strontium (hexafluoroacetylacetonate)2·tetraglyme. SBN thin films with compositions across the entire solid solution range were deposited. The nonlinear optical properties of the SBN films were also measured. Nonlinear optical coefficients approaching bulk values were obtained for as-deposited oriented films. The room temperature, effective second-order nonlinear coefficient was 3.0 pm/V. Films with the highest degree of crystalline perfection had the largest effective nonlinear coefficient. The second harmonic intensity was strongly temperature dependent with a maximum at the ferroelectric transition.",

author = "Nystrom, {M. J.} and Wessels, {B. W.} and Neumayer, {D. A.} and Marks, {Tobin J} and Lin, {W. P.} and Wong, {G. K.}",

year = "1995",

language = "English",

volume = "361",

pages = "167--172",

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publisher = "Materials Research Society",

note = "Proceedings of the 1994 MRS Fall Meeting ; Conference date: 29-11-1994 Through 02-12-1994",

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T1 - Deposition of strontium barium niobate thin films by metal-organic chemical vapor deposition and their nonlinear optical properties

AU - Nystrom, M. J.

AU - Wessels, B. W.

AU - Neumayer, D. A.

AU - Marks, Tobin J

AU - Lin, W. P.

AU - Wong, G. K.

PY - 1995

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N2 - Single phase, highly textured strontium barium niobate (SBN) thin films were deposited by low pressure metal-organic chemical vapor deposition on both crystalline and amorphous substrates. The metal precursors employed were niobium pentaethoxide as well as barium and strontium (hexafluoroacetylacetonate)2·tetraglyme. SBN thin films with compositions across the entire solid solution range were deposited. The nonlinear optical properties of the SBN films were also measured. Nonlinear optical coefficients approaching bulk values were obtained for as-deposited oriented films. The room temperature, effective second-order nonlinear coefficient was 3.0 pm/V. Films with the highest degree of crystalline perfection had the largest effective nonlinear coefficient. The second harmonic intensity was strongly temperature dependent with a maximum at the ferroelectric transition.

AB - Single phase, highly textured strontium barium niobate (SBN) thin films were deposited by low pressure metal-organic chemical vapor deposition on both crystalline and amorphous substrates. The metal precursors employed were niobium pentaethoxide as well as barium and strontium (hexafluoroacetylacetonate)2·tetraglyme. SBN thin films with compositions across the entire solid solution range were deposited. The nonlinear optical properties of the SBN films were also measured. Nonlinear optical coefficients approaching bulk values were obtained for as-deposited oriented films. The room temperature, effective second-order nonlinear coefficient was 3.0 pm/V. Films with the highest degree of crystalline perfection had the largest effective nonlinear coefficient. The second harmonic intensity was strongly temperature dependent with a maximum at the ferroelectric transition.

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