Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins

Thea M. Wilson, Torek A. Zeidan, Mahesh Hariharan, Frederick D. Lewis, Michael R Wasielewski

Research output: Contribution to journalArticle

51 Citations (Scopus)

Abstract

(Figure Presented) Charge on through: Perylenediimide chromophores incorporated into DNA hairpins serve as base-pair surrogates and form a zipperlike intercalated structure (see picture). Electron hopping was observed within the chromophore stacks upon one-electron reduction.

Original languageEnglish
Pages (from-to)2385-2388
Number of pages4
JournalAngewandte Chemie - International Edition
Volume49
Issue number13
Publication statusPublished - Mar 22 2010

Fingerprint

Chromophores
DNA
Electrons
Base Pairing
perylenediimide

Keywords

  • Chromophores
  • DNA
  • Electron transport
  • ENDOR spectroscopy
  • EPR spectroscopy

ASJC Scopus subject areas

  • Chemistry(all)
  • Catalysis
  • Medicine(all)

Cite this

Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins. / Wilson, Thea M.; Zeidan, Torek A.; Hariharan, Mahesh; Lewis, Frederick D.; Wasielewski, Michael R.

In: Angewandte Chemie - International Edition, Vol. 49, No. 13, 22.03.2010, p. 2385-2388.

Research output: Contribution to journalArticle

Wilson, Thea M. ; Zeidan, Torek A. ; Hariharan, Mahesh ; Lewis, Frederick D. ; Wasielewski, Michael R. / Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins. In: Angewandte Chemie - International Edition. 2010 ; Vol. 49, No. 13. pp. 2385-2388.
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