Enhanced Structural Stability and Photo Responsiveness of CH3NH3SnI3Perovskite via Pressure-Induced Amorphization and Recrystallization

Xujie Lü, Yonggang Wang, Constantinos C. Stoumpos, Qingyang Hu, Xiaofeng Guo, Haijie Chen, Liuxiang Yang, Jesse S. Smith, Wenge Yang, Yusheng Zhao, Hongwu Xu, Mercouri G. Kanatzidis, Quanxi Jia

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74 Citations (Scopus)

Abstract

Researchers compare the structural stability, electrical conductivity, and photo responsiveness of a lead-free tin halide perovskite CH3NH3SnI3 before and after high-pressure treatments up to 30 GPa. The pressure-driven phase transitions and evolution of associated electrical and optoelectronic properties have been characterized by in situ synchrotron X-ray diffraction (XRD), Raman spectroscopy, electrical resistance, and photocurrent measurements during two sequential compression and decompression cycles.

Original languageEnglish
Pages (from-to)8663-8668
Number of pages6
JournalAdvanced Materials
Volume28
Issue number39
DOIs
Publication statusPublished - 2016

Keywords

  • conductivity
  • enhanced photo responsiveness
  • high-pressure induced amorphization, recrystallization
  • organic–inorganic halide perovskites
  • stability

ASJC Scopus subject areas

  • Materials Science(all)
  • Mechanics of Materials
  • Mechanical Engineering

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    Lü, X., Wang, Y., Stoumpos, C. C., Hu, Q., Guo, X., Chen, H., Yang, L., Smith, J. S., Yang, W., Zhao, Y., Xu, H., Kanatzidis, M. G., & Jia, Q. (2016). Enhanced Structural Stability and Photo Responsiveness of CH3NH3SnI3Perovskite via Pressure-Induced Amorphization and Recrystallization. Advanced Materials, 28(39), 8663-8668. https://doi.org/10.1002/adma.201600771