Focused scattering of low energy Li+ from Mo(001): Experimental and computer simulation results

S. H. Overbury; P. C. Stair; P. A. Agron

doi:10.1016/0039-6028(83)90573-3

Focused scattering of low energy Li⁺ from Mo(001): Experimental and computer simulation results

S. H. Overbury, P. C. Stair, P. A. Agron

Northwestern University

Research output: Contribution to journal › Article › peer-review

18 Citations (Scopus)

Abstract

The azimuthal dependence of the energy distribution of Li⁺, specularly scattered from Mo(001), has been obtained for several incident energies E_i. The energy distributions exhibit one or two peaks, which always lie below the kinematical single scattering energy and which have intensity and energy that depend upon the azimuth. Due to trajectory focusing, the intensity is strongly peaked along the [100] azimuth for E_i ≲ 500 eV, but at higher E_i the intensity enhancement is shifted toward the [310] azimuth. Results of computer simulation give reasonable agreement with experimental observations. Analysis of the simulated trajectories allows identification of the scattering mechanisms which contribute to each portion of the spectrum.

Original language	English
Pages (from-to)	377-395
Number of pages	19
Journal	Surface Science
Volume	125
Issue number	2
DOIs	https://doi.org/10.1016/0039-6028(83)90573-3
Publication status	Published - Feb 2 1983

ASJC Scopus subject areas

Condensed Matter Physics
Surfaces and Interfaces
Surfaces, Coatings and Films
Materials Chemistry

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title = "Focused scattering of low energy Li+ from Mo(001): Experimental and computer simulation results",

abstract = "The azimuthal dependence of the energy distribution of Li+, specularly scattered from Mo(001), has been obtained for several incident energies Ei. The energy distributions exhibit one or two peaks, which always lie below the kinematical single scattering energy and which have intensity and energy that depend upon the azimuth. Due to trajectory focusing, the intensity is strongly peaked along the [100] azimuth for Ei ≲ 500 eV, but at higher Ei the intensity enhancement is shifted toward the [310] azimuth. Results of computer simulation give reasonable agreement with experimental observations. Analysis of the simulated trajectories allows identification of the scattering mechanisms which contribute to each portion of the spectrum.",

author = "Overbury, {S. H.} and Stair, {P. C.} and Agron, {P. A.}",

note = "Funding Information: sponsored by the Division of Chemical Sciences, Office of Basic Energy Sciences, US of Energy, under contract W-7405eng-26 with the Union Carbide Corporation. of Chemistry, Northwestern University, Evanston, Illinois 60201, USA.",

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T2 - Experimental and computer simulation results

AU - Overbury, S. H.

AU - Stair, P. C.

AU - Agron, P. A.

N1 - Funding Information: sponsored by the Division of Chemical Sciences, Office of Basic Energy Sciences, US of Energy, under contract W-7405eng-26 with the Union Carbide Corporation. of Chemistry, Northwestern University, Evanston, Illinois 60201, USA.

PY - 1983/2/2

Y1 - 1983/2/2

N2 - The azimuthal dependence of the energy distribution of Li+, specularly scattered from Mo(001), has been obtained for several incident energies Ei. The energy distributions exhibit one or two peaks, which always lie below the kinematical single scattering energy and which have intensity and energy that depend upon the azimuth. Due to trajectory focusing, the intensity is strongly peaked along the [100] azimuth for Ei ≲ 500 eV, but at higher Ei the intensity enhancement is shifted toward the [310] azimuth. Results of computer simulation give reasonable agreement with experimental observations. Analysis of the simulated trajectories allows identification of the scattering mechanisms which contribute to each portion of the spectrum.

AB - The azimuthal dependence of the energy distribution of Li+, specularly scattered from Mo(001), has been obtained for several incident energies Ei. The energy distributions exhibit one or two peaks, which always lie below the kinematical single scattering energy and which have intensity and energy that depend upon the azimuth. Due to trajectory focusing, the intensity is strongly peaked along the [100] azimuth for Ei ≲ 500 eV, but at higher Ei the intensity enhancement is shifted toward the [310] azimuth. Results of computer simulation give reasonable agreement with experimental observations. Analysis of the simulated trajectories allows identification of the scattering mechanisms which contribute to each portion of the spectrum.

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