Hyper-Rayleigh scattering from silver nanoparticles

E. C. Hao, George C Schatz, R. C. Johnson, Joseph T Hupp

Research output: Contribution to journalArticle

110 Citations (Scopus)

Abstract

A study was conducted on the leading-order contribution to the incoherent second harmonic generation of silver nanoparticles. By measuring the excitation wavelength dependence of βsilver, distinguishable dipole and quadrupole plasmon contributions to hyper-Rayleigh intensities were experimentally demonstrated. These two contributions have different angular distributions, and it was shown that DSEH theory in conjunction with simple angular distribution measurements may be used to determine the relative sizes of the dipole and quadrupole contributions.

Original languageEnglish
Pages (from-to)5963-5966
Number of pages4
JournalJournal of Chemical Physics
Volume117
Issue number13
DOIs
Publication statusPublished - Oct 1 2002

Fingerprint

Rayleigh scattering
Angular distribution
Silver
angular distribution
quadrupoles
silver
dipoles
Nanoparticles
nanoparticles
Harmonic generation
harmonic generations
Wavelength
wavelengths
excitation

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

Cite this

Hyper-Rayleigh scattering from silver nanoparticles. / Hao, E. C.; Schatz, George C; Johnson, R. C.; Hupp, Joseph T.

In: Journal of Chemical Physics, Vol. 117, No. 13, 01.10.2002, p. 5963-5966.

Research output: Contribution to journalArticle

Hao, E. C. ; Schatz, George C ; Johnson, R. C. ; Hupp, Joseph T. / Hyper-Rayleigh scattering from silver nanoparticles. In: Journal of Chemical Physics. 2002 ; Vol. 117, No. 13. pp. 5963-5966.
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