Abstract
An attractive and challenging approach to the construction of robust, structurally precise thin film materials with large second-order optical nonlinearities or electroluminescent characteristics is the covalent self-assembly of arrays of tailored molecular building blocks. In this contribution, we discuss the implementation of self-limiting siloxane self-assembly processes to achieve the fabrication of structurally regular organic LED (OLED) devices. Areas surveyed include: i) the use of layer-by-layer self-assembly for ITO electrode modification/passivation/hole-electron carrier balancing in vapor depositied devices, ii) the synthesis of chlorosilane-functionalized precursor molecules for hole transport (HTL), emissive layer (EML), and electron transport layer (ETL) self-assembly, iii) the physicochemical and microstructural characterization of the HTL self-assembly process employing a triarylamine precursor, iv) the fabrication and characterization of a hybrid self-assembled + vapor deposited two-layer OLED, v) the fabrication and characterization of a fully self-assembled two-layer OLED.
| Original language | English |
|---|---|
| Title of host publication | Proceedings of SPIE - The International Society for Optical Engineering |
| Editors | B Kippelen, D.D.C. Bradley |
| Pages | 148-155 |
| Number of pages | 8 |
| Volume | 3281 |
| DOIs | |
| Publication status | Published - 1998 |
| Event | Polymer Photonic Devices - San Jose, CA, United States Duration: Jan 28 1998 → Jan 30 1998 |
Other
| Other | Polymer Photonic Devices |
|---|---|
| Country | United States |
| City | San Jose, CA |
| Period | 1/28/98 → 1/30/98 |
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Keywords
- Electroluminescent device
- Organic LED
- Self-assembly
- Thin film LED
ASJC Scopus subject areas
- Electrical and Electronic Engineering
- Condensed Matter Physics
Cite this
Molecular self-assembly approaches to multilayer organic light-emitting diode structures. / Malinsky, Joshua E.; Li, Weijin; Chou, Homer; Ma, Wuping; Geng, Lifeng; Marks, Tobin J; Jabbour, Ghassan E.; Shaheen, Sean E.; Kippelen, Bernard; Peyghambarian, Nasser; Dutta, Pulak; Richter, Andrew J.; Armstrong, Neal R.; Lee, Paul A.; Anderson, Jeffrey D.
Proceedings of SPIE - The International Society for Optical Engineering. ed. / B Kippelen; D.D.C. Bradley. Vol. 3281 1998. p. 148-155.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution
}
TY - GEN
T1 - Molecular self-assembly approaches to multilayer organic light-emitting diode structures
AU - Malinsky, Joshua E.
AU - Li, Weijin
AU - Chou, Homer
AU - Ma, Wuping
AU - Geng, Lifeng
AU - Marks, Tobin J
AU - Jabbour, Ghassan E.
AU - Shaheen, Sean E.
AU - Kippelen, Bernard
AU - Peyghambarian, Nasser
AU - Dutta, Pulak
AU - Richter, Andrew J.
AU - Armstrong, Neal R.
AU - Lee, Paul A.
AU - Anderson, Jeffrey D.
PY - 1998
Y1 - 1998
N2 - An attractive and challenging approach to the construction of robust, structurally precise thin film materials with large second-order optical nonlinearities or electroluminescent characteristics is the covalent self-assembly of arrays of tailored molecular building blocks. In this contribution, we discuss the implementation of self-limiting siloxane self-assembly processes to achieve the fabrication of structurally regular organic LED (OLED) devices. Areas surveyed include: i) the use of layer-by-layer self-assembly for ITO electrode modification/passivation/hole-electron carrier balancing in vapor depositied devices, ii) the synthesis of chlorosilane-functionalized precursor molecules for hole transport (HTL), emissive layer (EML), and electron transport layer (ETL) self-assembly, iii) the physicochemical and microstructural characterization of the HTL self-assembly process employing a triarylamine precursor, iv) the fabrication and characterization of a hybrid self-assembled + vapor deposited two-layer OLED, v) the fabrication and characterization of a fully self-assembled two-layer OLED.
AB - An attractive and challenging approach to the construction of robust, structurally precise thin film materials with large second-order optical nonlinearities or electroluminescent characteristics is the covalent self-assembly of arrays of tailored molecular building blocks. In this contribution, we discuss the implementation of self-limiting siloxane self-assembly processes to achieve the fabrication of structurally regular organic LED (OLED) devices. Areas surveyed include: i) the use of layer-by-layer self-assembly for ITO electrode modification/passivation/hole-electron carrier balancing in vapor depositied devices, ii) the synthesis of chlorosilane-functionalized precursor molecules for hole transport (HTL), emissive layer (EML), and electron transport layer (ETL) self-assembly, iii) the physicochemical and microstructural characterization of the HTL self-assembly process employing a triarylamine precursor, iv) the fabrication and characterization of a hybrid self-assembled + vapor deposited two-layer OLED, v) the fabrication and characterization of a fully self-assembled two-layer OLED.
KW - Electroluminescent device
KW - Organic LED
KW - Self-assembly
KW - Thin film LED
UR - http://www.scopus.com/inward/record.url?scp=0012356789&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=0012356789&partnerID=8YFLogxK
U2 - 10.1117/12.305415
DO - 10.1117/12.305415
M3 - Conference contribution
AN - SCOPUS:0012356789
VL - 3281
SP - 148
EP - 155
BT - Proceedings of SPIE - The International Society for Optical Engineering
A2 - Kippelen, B
A2 - Bradley, D.D.C.
ER -