Abstract
A new strategy to achieve high NO removal at low temperatures in an oxygen rich atmosphere is studied. This approach involves a coupled system: an ethylene glycol (EG) reforming unit to convert a mixture of ethylene glycol and water into hydrogen and CO followed by a H2-deNOx unit. The performance of modified Pt supported catalyst for gas phase EG reforming at 230°C was examined. Prior to testing, the samples were calcined in air followed by reduction in H2 at 250°C. Modification of the Pt supported catalysts with Na produce a twofold effect, an increase in the reforming activity and also stability of the catalyst. At 420 ppm EG concentration, results indicate complete conversion of ethylene glycol into hydrogen, mainly via decomposition. At higher EG concentrations (2.15% EG in the feed), oxidative reforming produced 1.4 H2/EG. This EG reforming unit is coupled to a de-NOx unit. Based on calculations, 0.551 kg of reforming catalyst would be needed to deliver the amount of H2 for complete NOx removal. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).
| Original language | English |
|---|---|
| Title of host publication | AIChE Annual Meeting Conference Proceedings |
| Publisher | American Institute of Chemical Engineers |
| Volume | 2005 |
| ISBN (Print) | 0816909962, 9780816909964 |
| Publication status | Published - 2005 |
| Event | 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase - Cincinnati, OH, United States Duration: Oct 30 2005 → Nov 4 2005 |
Other
| Other | 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase |
|---|---|
| Country | United States |
| City | Cincinnati, OH |
| Period | 10/30/05 → 11/4/05 |
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ASJC Scopus subject areas
- Energy(all)
Cite this
Novel low temperature Nox removal for diesel exhaust. / Law, Hiu Ying; Kung, Mayfair C.; Kung, Harold H.
AIChE Annual Meeting Conference Proceedings. Vol. 2005 American Institute of Chemical Engineers, 2005.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution
}
TY - GEN
T1 - Novel low temperature Nox removal for diesel exhaust
AU - Law, Hiu Ying
AU - Kung, Mayfair C.
AU - Kung, Harold H
PY - 2005
Y1 - 2005
N2 - A new strategy to achieve high NO removal at low temperatures in an oxygen rich atmosphere is studied. This approach involves a coupled system: an ethylene glycol (EG) reforming unit to convert a mixture of ethylene glycol and water into hydrogen and CO followed by a H2-deNOx unit. The performance of modified Pt supported catalyst for gas phase EG reforming at 230°C was examined. Prior to testing, the samples were calcined in air followed by reduction in H2 at 250°C. Modification of the Pt supported catalysts with Na produce a twofold effect, an increase in the reforming activity and also stability of the catalyst. At 420 ppm EG concentration, results indicate complete conversion of ethylene glycol into hydrogen, mainly via decomposition. At higher EG concentrations (2.15% EG in the feed), oxidative reforming produced 1.4 H2/EG. This EG reforming unit is coupled to a de-NOx unit. Based on calculations, 0.551 kg of reforming catalyst would be needed to deliver the amount of H2 for complete NOx removal. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).
AB - A new strategy to achieve high NO removal at low temperatures in an oxygen rich atmosphere is studied. This approach involves a coupled system: an ethylene glycol (EG) reforming unit to convert a mixture of ethylene glycol and water into hydrogen and CO followed by a H2-deNOx unit. The performance of modified Pt supported catalyst for gas phase EG reforming at 230°C was examined. Prior to testing, the samples were calcined in air followed by reduction in H2 at 250°C. Modification of the Pt supported catalysts with Na produce a twofold effect, an increase in the reforming activity and also stability of the catalyst. At 420 ppm EG concentration, results indicate complete conversion of ethylene glycol into hydrogen, mainly via decomposition. At higher EG concentrations (2.15% EG in the feed), oxidative reforming produced 1.4 H2/EG. This EG reforming unit is coupled to a de-NOx unit. Based on calculations, 0.551 kg of reforming catalyst would be needed to deliver the amount of H2 for complete NOx removal. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).
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UR - http://www.scopus.com/inward/citedby.url?scp=84916885941&partnerID=8YFLogxK
M3 - Conference contribution
AN - SCOPUS:84916885941
SN - 0816909962
SN - 9780816909964
VL - 2005
BT - AIChE Annual Meeting Conference Proceedings
PB - American Institute of Chemical Engineers
ER -