Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite

David A. Valverde-Chavez, Carlito S. Ponseca, Constantinos Stoumpos, Arkady Yartsev, Mercouri G Kanatzidis, Villy Sundstrom, David G. Cooke

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

We analyzed ultrafast photocarrier generation in single crystal CH3NH3PbI3 perovskite through time-resolved terahertz spectroscopy. We find a Drude-Lorentz type conductivity spectra with a carrier mobility of 35 cm2/Vs and a Lorentzian component at 45 meV possibly due to intra-excitonic transitions.

Original languageEnglish
Title of host publicationConference on Lasers and Electro-Optics Europe - Technical Digest
PublisherInstitute of Electrical and Electronics Engineers Inc.
Volume2015-August
ISBN (Print)9781557529688
Publication statusPublished - Aug 10 2015
EventConference on Lasers and Electro-Optics, CLEO 2015 - San Jose, United States
Duration: May 10 2015May 15 2015

Other

OtherConference on Lasers and Electro-Optics, CLEO 2015
CountryUnited States
CitySan Jose
Period5/10/155/15/15

Fingerprint

Terahertz spectroscopy
Carrier mobility
carrier mobility
Perovskite
halides
Lead
Single crystals
Pumps
Spectroscopy
pumps
conductivity
probes
single crystals
spectroscopy
perovskite

Keywords

  • Conductivity
  • Crystals
  • Laser beams
  • Laser excitation
  • Particle beams
  • Probes
  • Spectroscopy

ASJC Scopus subject areas

  • Electrical and Electronic Engineering
  • Atomic and Molecular Physics, and Optics
  • Electronic, Optical and Magnetic Materials

Cite this

Valverde-Chavez, D. A., Ponseca, C. S., Stoumpos, C., Yartsev, A., Kanatzidis, M. G., Sundstrom, V., & Cooke, D. G. (2015). Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite. In Conference on Lasers and Electro-Optics Europe - Technical Digest (Vol. 2015-August). [7183638] Institute of Electrical and Electronics Engineers Inc..

Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite. / Valverde-Chavez, David A.; Ponseca, Carlito S.; Stoumpos, Constantinos; Yartsev, Arkady; Kanatzidis, Mercouri G; Sundstrom, Villy; Cooke, David G.

Conference on Lasers and Electro-Optics Europe - Technical Digest. Vol. 2015-August Institute of Electrical and Electronics Engineers Inc., 2015. 7183638.

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Valverde-Chavez, DA, Ponseca, CS, Stoumpos, C, Yartsev, A, Kanatzidis, MG, Sundstrom, V & Cooke, DG 2015, Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite. in Conference on Lasers and Electro-Optics Europe - Technical Digest. vol. 2015-August, 7183638, Institute of Electrical and Electronics Engineers Inc., Conference on Lasers and Electro-Optics, CLEO 2015, San Jose, United States, 5/10/15.
Valverde-Chavez DA, Ponseca CS, Stoumpos C, Yartsev A, Kanatzidis MG, Sundstrom V et al. Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite. In Conference on Lasers and Electro-Optics Europe - Technical Digest. Vol. 2015-August. Institute of Electrical and Electronics Engineers Inc. 2015. 7183638
Valverde-Chavez, David A. ; Ponseca, Carlito S. ; Stoumpos, Constantinos ; Yartsev, Arkady ; Kanatzidis, Mercouri G ; Sundstrom, Villy ; Cooke, David G. / Optical pump - Multi-THz probe spectroscopy of a single crystal organic hybrid lead halide perovskite. Conference on Lasers and Electro-Optics Europe - Technical Digest. Vol. 2015-August Institute of Electrical and Electronics Engineers Inc., 2015.
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AU - Yartsev, Arkady

AU - Kanatzidis, Mercouri G

AU - Sundstrom, Villy

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