Photo-induced current transient spectroscopy of single crystal Tl6I4Se

Z. Liu, J. A. Peters, M. Sebastian, Mercouri G Kanatzidis, J. Im, Arthur J Freeman, B. W. Wessels

Research output: Contribution to journalArticle

6 Citations (Scopus)

Abstract

The compound Tl6I4Se is a promising wide band gap semiconductor for hard radiation detection at room temperature. To further improve its detection efficiency, native defects have been investigated using photo-induced current transient spectroscopy (PICTS). We observe two shallow acceptor levels with mean activation energies of 76, 175 meV, and two shallow donor defects 62, and 96 meV, respectively. No deeper donor levels are observed. The levels are attributed to native point defects. Defect capture cross sections in the range 10-21 to 10-18 cm2 were measured. The small capture cross sections are attributed to the effective screening of the defects due to a large static dielectric constant.

Original languageEnglish
Article number115002
JournalSemiconductor Science and Technology
Volume29
Issue number11
DOIs
Publication statusPublished - Nov 1 2014

Fingerprint

Induced currents
Single crystals
Spectroscopy
Defects
single crystals
defects
absorption cross sections
spectroscopy
Point defects
point defects
Screening
Permittivity
screening
Activation energy
permittivity
activation energy
broadband
Radiation
room temperature
radiation

Keywords

  • charge carriers: generation
  • lifetime and trapping
  • other semiconductors
  • photoconduction and photovoltaic effects
  • recombination

ASJC Scopus subject areas

  • Electrical and Electronic Engineering
  • Electronic, Optical and Magnetic Materials
  • Materials Chemistry
  • Condensed Matter Physics

Cite this

Photo-induced current transient spectroscopy of single crystal Tl6I4Se. / Liu, Z.; Peters, J. A.; Sebastian, M.; Kanatzidis, Mercouri G; Im, J.; Freeman, Arthur J; Wessels, B. W.

In: Semiconductor Science and Technology, Vol. 29, No. 11, 115002, 01.11.2014.

Research output: Contribution to journalArticle

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AU - Freeman, Arthur J

AU - Wessels, B. W.

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