Abstract
Three-dimensional dielectric photonic crystals have well-established enhanced light-matter interactions via high Q factors. Their plasmonic counterparts based on arrays of nanoparticles, however, have not been experimentally well explored owing to a lack of available synthetic routes for preparing them. However, such structures should facilitate these interactions based on the small mode volumes associated with plasmonic polarization. Herein we report strong light-plasmon interactions within 3D plasmonic photonic crystals that have lattice constants and nanoparticle diameters that can be independently controlled in the deep subwavelength size regime by using a DNA-programmable assembly technique. The strong coupling within such crystals is probed with backscattering spectra, and the mode splitting (0.10 and 0.24 eV) is defined based on dispersion diagrams. Numerical simulations predict that the crystal photonic modes (Fabry-Perot modes) can be enhanced by coating the crystals with a silver layer, achieving moderate Q factors (∼102) over the visible and near-infrared spectrum.
| Original language | English |
|---|---|
| Pages (from-to) | 977-981 |
| Number of pages | 5 |
| Journal | Proceedings of the National Academy of Sciences of the United States of America |
| Volume | 112 |
| Issue number | 4 |
| DOIs | |
| Publication status | Published - Jan 27 2015 |
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Keywords
- 3D photonic crystals
- Deep subwavelength scale
- DNA-programmable assembly
- Plasmonics
- Strong coupling
ASJC Scopus subject areas
- General
Cite this
Plasmonic photonic crystals realized through DNA-programmable assembly. / Park, Daniel J.; Zhang, Chuan; Ku, Jessie C.; Zhou, Yu; Schatz, George C; Mirkin, Chad A.
In: Proceedings of the National Academy of Sciences of the United States of America, Vol. 112, No. 4, 27.01.2015, p. 977-981.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Plasmonic photonic crystals realized through DNA-programmable assembly
AU - Park, Daniel J.
AU - Zhang, Chuan
AU - Ku, Jessie C.
AU - Zhou, Yu
AU - Schatz, George C
AU - Mirkin, Chad A.
PY - 2015/1/27
Y1 - 2015/1/27
N2 - Three-dimensional dielectric photonic crystals have well-established enhanced light-matter interactions via high Q factors. Their plasmonic counterparts based on arrays of nanoparticles, however, have not been experimentally well explored owing to a lack of available synthetic routes for preparing them. However, such structures should facilitate these interactions based on the small mode volumes associated with plasmonic polarization. Herein we report strong light-plasmon interactions within 3D plasmonic photonic crystals that have lattice constants and nanoparticle diameters that can be independently controlled in the deep subwavelength size regime by using a DNA-programmable assembly technique. The strong coupling within such crystals is probed with backscattering spectra, and the mode splitting (0.10 and 0.24 eV) is defined based on dispersion diagrams. Numerical simulations predict that the crystal photonic modes (Fabry-Perot modes) can be enhanced by coating the crystals with a silver layer, achieving moderate Q factors (∼102) over the visible and near-infrared spectrum.
AB - Three-dimensional dielectric photonic crystals have well-established enhanced light-matter interactions via high Q factors. Their plasmonic counterparts based on arrays of nanoparticles, however, have not been experimentally well explored owing to a lack of available synthetic routes for preparing them. However, such structures should facilitate these interactions based on the small mode volumes associated with plasmonic polarization. Herein we report strong light-plasmon interactions within 3D plasmonic photonic crystals that have lattice constants and nanoparticle diameters that can be independently controlled in the deep subwavelength size regime by using a DNA-programmable assembly technique. The strong coupling within such crystals is probed with backscattering spectra, and the mode splitting (0.10 and 0.24 eV) is defined based on dispersion diagrams. Numerical simulations predict that the crystal photonic modes (Fabry-Perot modes) can be enhanced by coating the crystals with a silver layer, achieving moderate Q factors (∼102) over the visible and near-infrared spectrum.
KW - 3D photonic crystals
KW - Deep subwavelength scale
KW - DNA-programmable assembly
KW - Plasmonics
KW - Strong coupling
UR - http://www.scopus.com/inward/record.url?scp=84921992081&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84921992081&partnerID=8YFLogxK
U2 - 10.1073/pnas.1422649112
DO - 10.1073/pnas.1422649112
M3 - Article
C2 - 25548175
AN - SCOPUS:84921992081
VL - 112
SP - 977
EP - 981
JO - Proceedings of the National Academy of Sciences of the United States of America
JF - Proceedings of the National Academy of Sciences of the United States of America
SN - 0027-8424
IS - 4
ER -