Abstract
This paper reports how geometric effects in low-symmetry plasmonic nanoparticle arrays can produce polarization-dependent lasing responses. We developed a scalable fabrication procedure to pattern rhombohedral arrays of aluminum anisotropic nanoparticles that support lattice plasmon modes from both first-order and second-order diffraction coupling. We found that nanoparticle shape can be used to engineer the spatial overlap between electromagnetic hot spots of different lattice modes and dye gain to support plasmonic lasing. The lasing behavior revealed that plasmon-exciton energy transfer depends on polarization, with stronger coupling and faster dynamics when the transition dipole moments of the excited gain are aligned with the electric field of the plasmon modes.
| Original language | English |
|---|---|
| Pages (from-to) | 7435-7441 |
| Number of pages | 7 |
| Journal | ACS nano |
| Volume | 13 |
| Issue number | 7 |
| DOIs | |
| Publication status | Published - Jul 23 2019 |
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Keywords
- Aluminum plasmonics
- Anisotropic nanoparticles
- Lasing
- Lattice plasmons
- Polarization
- Symmetry
ASJC Scopus subject areas
- Materials Science(all)
- Engineering(all)
- Physics and Astronomy(all)
Cite this
Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays. / Knudson, Michael P.; Li, Ran; Wang, Danqing; Wang, Weijia; Schaller, Richard D; Odom, Teri W.
In: ACS nano, Vol. 13, No. 7, 23.07.2019, p. 7435-7441.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays
AU - Knudson, Michael P.
AU - Li, Ran
AU - Wang, Danqing
AU - Wang, Weijia
AU - Schaller, Richard D
AU - Odom, Teri W
PY - 2019/7/23
Y1 - 2019/7/23
N2 - This paper reports how geometric effects in low-symmetry plasmonic nanoparticle arrays can produce polarization-dependent lasing responses. We developed a scalable fabrication procedure to pattern rhombohedral arrays of aluminum anisotropic nanoparticles that support lattice plasmon modes from both first-order and second-order diffraction coupling. We found that nanoparticle shape can be used to engineer the spatial overlap between electromagnetic hot spots of different lattice modes and dye gain to support plasmonic lasing. The lasing behavior revealed that plasmon-exciton energy transfer depends on polarization, with stronger coupling and faster dynamics when the transition dipole moments of the excited gain are aligned with the electric field of the plasmon modes.
AB - This paper reports how geometric effects in low-symmetry plasmonic nanoparticle arrays can produce polarization-dependent lasing responses. We developed a scalable fabrication procedure to pattern rhombohedral arrays of aluminum anisotropic nanoparticles that support lattice plasmon modes from both first-order and second-order diffraction coupling. We found that nanoparticle shape can be used to engineer the spatial overlap between electromagnetic hot spots of different lattice modes and dye gain to support plasmonic lasing. The lasing behavior revealed that plasmon-exciton energy transfer depends on polarization, with stronger coupling and faster dynamics when the transition dipole moments of the excited gain are aligned with the electric field of the plasmon modes.
KW - Aluminum plasmonics
KW - Anisotropic nanoparticles
KW - Lasing
KW - Lattice plasmons
KW - Polarization
KW - Symmetry
UR - http://www.scopus.com/inward/record.url?scp=85070421817&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85070421817&partnerID=8YFLogxK
U2 - 10.1021/acsnano.9b01142
DO - 10.1021/acsnano.9b01142
M3 - Article
C2 - 30938987
AN - SCOPUS:85070421817
VL - 13
SP - 7435
EP - 7441
JO - ACS Nano
JF - ACS Nano
SN - 1936-0851
IS - 7
ER -