Pressure effects on interfacial surface contacts and performance of organic solar cells

B. Agyei-Tuffour, N. Y. Doumon, E. R. Rwenyagila, J. Asare, O. K. Oyewole, Z. Shen, C. E. Petoukhoff, M. G. Zebaze Kana, Deirdre M O'Carroll, W. O. Soboyejo

Research output: Contribution to journalArticle

Abstract

This paper explores the effects of pressure on the interfacial surface contacts and the performance of organic solar cells. A combination of experimental techniques and analytical/computational models is used to study the evolving surface contacts profiles that occur when compliant, semi-rigid and rigid particles are interlocked between adjacent layers in model solar cell structures. The effects of layer surface roughness and interlocked (trapped) particles are also considered along with the effects of surface energy, adhesion energy, and pressure. The results show that increased interfacial contact lengths and decreased void lengths are associated with the application of increased pressure. Increased pressure also results in significant improvements in power conversion efficiency. These improvements in power conversion efficiency are associated with the closure up of micro- and nano-voids due to the application of pressure to layers produced via spin coating and thermal evaporation. The results suggest that pressure-induced contacts can be used to enhance the performance of organic solar cells.

Original languageEnglish
Article number205501
JournalJournal of Applied Physics
Volume122
Issue number20
DOIs
Publication statusPublished - Nov 28 2017

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pressure effects
solar cells
voids
trapped particles
closures
surface energy
coating
surface roughness
adhesion
evaporation
profiles

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Agyei-Tuffour, B., Doumon, N. Y., Rwenyagila, E. R., Asare, J., Oyewole, O. K., Shen, Z., ... Soboyejo, W. O. (2017). Pressure effects on interfacial surface contacts and performance of organic solar cells. Journal of Applied Physics, 122(20), [205501]. https://doi.org/10.1063/1.5001765

Pressure effects on interfacial surface contacts and performance of organic solar cells. / Agyei-Tuffour, B.; Doumon, N. Y.; Rwenyagila, E. R.; Asare, J.; Oyewole, O. K.; Shen, Z.; Petoukhoff, C. E.; Zebaze Kana, M. G.; O'Carroll, Deirdre M; Soboyejo, W. O.

In: Journal of Applied Physics, Vol. 122, No. 20, 205501, 28.11.2017.

Research output: Contribution to journalArticle

Agyei-Tuffour, B, Doumon, NY, Rwenyagila, ER, Asare, J, Oyewole, OK, Shen, Z, Petoukhoff, CE, Zebaze Kana, MG, O'Carroll, DM & Soboyejo, WO 2017, 'Pressure effects on interfacial surface contacts and performance of organic solar cells', Journal of Applied Physics, vol. 122, no. 20, 205501. https://doi.org/10.1063/1.5001765
Agyei-Tuffour B, Doumon NY, Rwenyagila ER, Asare J, Oyewole OK, Shen Z et al. Pressure effects on interfacial surface contacts and performance of organic solar cells. Journal of Applied Physics. 2017 Nov 28;122(20). 205501. https://doi.org/10.1063/1.5001765
Agyei-Tuffour, B. ; Doumon, N. Y. ; Rwenyagila, E. R. ; Asare, J. ; Oyewole, O. K. ; Shen, Z. ; Petoukhoff, C. E. ; Zebaze Kana, M. G. ; O'Carroll, Deirdre M ; Soboyejo, W. O. / Pressure effects on interfacial surface contacts and performance of organic solar cells. In: Journal of Applied Physics. 2017 ; Vol. 122, No. 20.
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