Abstract
Quantum control of coherent anti-Stokes Raman spectroscopy (CARS) was demonstrated. Raman spectra was measured with a resolution of the order of 5 cm-1 using shaped pulses with a bandwidth of about 120 cm-1. Nearly complete suppression of the nonresonant background signal was also demonstrated. Selective population of only one of the two Raman levels of pyridine, lying within the bandwidth of excitation pulses, was achieved. Simple modeling was used to derive the required spectral phases and the measured signals were found in agreement with the model predictions.
| Original language | English |
|---|---|
| Pages (from-to) | 434081-434084 |
| Number of pages | 4 |
| Journal | Physical Review A |
| Volume | 65 |
| Issue number | 4 B |
| Publication status | Published - Apr 2002 |
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ASJC Scopus subject areas
- Physics and Astronomy(all)
- Atomic and Molecular Physics, and Optics
Cite this
Quantum control of coherent anti-Stokes Raman processes. / Oron, Dan; Dudovich, Nirit; Yelin, Dvir; Silberberg, Yaron.
In: Physical Review A, Vol. 65, No. 4 B, 04.2002, p. 434081-434084.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Quantum control of coherent anti-Stokes Raman processes
AU - Oron, Dan
AU - Dudovich, Nirit
AU - Yelin, Dvir
AU - Silberberg, Yaron
PY - 2002/4
Y1 - 2002/4
N2 - Quantum control of coherent anti-Stokes Raman spectroscopy (CARS) was demonstrated. Raman spectra was measured with a resolution of the order of 5 cm-1 using shaped pulses with a bandwidth of about 120 cm-1. Nearly complete suppression of the nonresonant background signal was also demonstrated. Selective population of only one of the two Raman levels of pyridine, lying within the bandwidth of excitation pulses, was achieved. Simple modeling was used to derive the required spectral phases and the measured signals were found in agreement with the model predictions.
AB - Quantum control of coherent anti-Stokes Raman spectroscopy (CARS) was demonstrated. Raman spectra was measured with a resolution of the order of 5 cm-1 using shaped pulses with a bandwidth of about 120 cm-1. Nearly complete suppression of the nonresonant background signal was also demonstrated. Selective population of only one of the two Raman levels of pyridine, lying within the bandwidth of excitation pulses, was achieved. Simple modeling was used to derive the required spectral phases and the measured signals were found in agreement with the model predictions.
UR - http://www.scopus.com/inward/record.url?scp=0036542174&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=0036542174&partnerID=8YFLogxK
M3 - Article
VL - 65
SP - 434081
EP - 434084
JO - Physical Review A - Atomic, Molecular, and Optical Physics
JF - Physical Review A - Atomic, Molecular, and Optical Physics
SN - 1050-2947
IS - 4 B
ER -