Abstract
Using femtosecond pulse-shaping techniques, we are able to control several useful parameters of coherent anti-Stokes Raman spectroscopy (CARS). By shaping both the pump and the Stokes pulses with an appropriate spectral phase function, we eliminated the nonresonant CARS background. In addition, we designed pulses which selectively excite one of two neighboring Raman levels, even when both are well within the excitation spectrum. High-resolution CARS spectra were recorded in spite of the broad femtosecond pulse spectrum.
| Original language | English |
|---|---|
| Number of pages | 1 |
| Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
| Volume | 65 |
| Issue number | 4 |
| DOIs | |
| Publication status | Published - Jan 1 2002 |
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ASJC Scopus subject areas
- Atomic and Molecular Physics, and Optics
Cite this
Quantum control of coherent anti-Stokes Raman processes. / Oron, Dan; Dudovich, Nirit; Yelin, Dvir; Silberberg, Yaron.
In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 65, No. 4, 01.01.2002.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Quantum control of coherent anti-Stokes Raman processes
AU - Oron, Dan
AU - Dudovich, Nirit
AU - Yelin, Dvir
AU - Silberberg, Yaron
PY - 2002/1/1
Y1 - 2002/1/1
N2 - Using femtosecond pulse-shaping techniques, we are able to control several useful parameters of coherent anti-Stokes Raman spectroscopy (CARS). By shaping both the pump and the Stokes pulses with an appropriate spectral phase function, we eliminated the nonresonant CARS background. In addition, we designed pulses which selectively excite one of two neighboring Raman levels, even when both are well within the excitation spectrum. High-resolution CARS spectra were recorded in spite of the broad femtosecond pulse spectrum.
AB - Using femtosecond pulse-shaping techniques, we are able to control several useful parameters of coherent anti-Stokes Raman spectroscopy (CARS). By shaping both the pump and the Stokes pulses with an appropriate spectral phase function, we eliminated the nonresonant CARS background. In addition, we designed pulses which selectively excite one of two neighboring Raman levels, even when both are well within the excitation spectrum. High-resolution CARS spectra were recorded in spite of the broad femtosecond pulse spectrum.
UR - http://www.scopus.com/inward/record.url?scp=14544301588&partnerID=8YFLogxK
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U2 - 10.1103/PhysRevA.65.043408
DO - 10.1103/PhysRevA.65.043408
M3 - Article
VL - 65
JO - Physical Review A
JF - Physical Review A
SN - 2469-9926
IS - 4
ER -