Quantum control of coherent anti-Stokes Raman processes

Dan Oron; Nirit Dudovich; Dvir Yelin; Yaron Silberberg

doi:10.1103/PhysRevA.65.043408

Quantum control of coherent anti-Stokes Raman processes

Dan Oron, Nirit Dudovich, Dvir Yelin, Yaron Silberberg

Weizmann Institute of Science, Israel

Research output: Contribution to journal › Article › peer-review

4 Citations (Scopus)

Abstract

Using femtosecond pulse-shaping techniques, we are able to control several useful parameters of coherent anti-Stokes Raman spectroscopy (CARS). By shaping both the pump and the Stokes pulses with an appropriate spectral phase function, we eliminated the nonresonant CARS background. In addition, we designed pulses which selectively excite one of two neighboring Raman levels, even when both are well within the excitation spectrum. High-resolution CARS spectra were recorded in spite of the broad femtosecond pulse spectrum.

Original language	English
Number of pages	1
Journal	Physical Review A - Atomic, Molecular, and Optical Physics
Volume	65
Issue number	4
DOIs	https://doi.org/10.1103/PhysRevA.65.043408
Publication status	Published - Jan 1 2002

ASJC Scopus subject areas

Atomic and Molecular Physics, and Optics

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