Quantum dynamics simulation of the ultrafast photoionization of Li2

Lorenzo Pesce, Zohar Amitay, Radoslaw Uberna, Stephen R. Leone, Mark Ratner, Ronnie Kosloff

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33 Citations (Scopus)

Abstract

The experimental pump/probe ultrafast photoionization of the lithium species were compared with the quantum dynamical calculations on potential energy surfaces. The perturbation techniques were used to analyze the quantum dynamics of signals obtained with different laser pulse shapes, intensities and chirps. The pumps show the inadequacies of the potential surfaces and dipole moment matrix elements of lithium dimer.

Original languageEnglish
Pages (from-to)1259-1271
Number of pages13
JournalJournal of Chemical Physics
Volume114
Issue number3
DOIs
Publication statusPublished - Jan 1 2001

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ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

Cite this

Pesce, L., Amitay, Z., Uberna, R., Leone, S. R., Ratner, M., & Kosloff, R. (2001). Quantum dynamics simulation of the ultrafast photoionization of Li2. Journal of Chemical Physics, 114(3), 1259-1271. https://doi.org/10.1063/1.1333004