Abstract
Single-pulse vibrational spectroscopy was readily achieved using coherent control techniques. By tailoring the spectral phase of an ultrashort pulse, the interference between quantum processes induced by the various spectral components of the pulse was controlled, leading either to selective population of given Raman levels or to the generation of narrow features in the CARS spectrum by all the populated Raman levels. By applying this principle, high-resolution spectroscopy was demonstrated in the vibrational energy range 700-1400 cm-1. By measuring a complex Raman spectrum of a molecule in this spectral region, the method was found to be robust and practical.
| Original language | English |
|---|---|
| Pages (from-to) | 9208-9215 |
| Number of pages | 8 |
| Journal | Journal of Chemical Physics |
| Volume | 118 |
| Issue number | 20 |
| DOIs | |
| Publication status | Published - May 22 2003 |
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ASJC Scopus subject areas
- Atomic and Molecular Physics, and Optics
Cite this
Single-pulse coherent anti-Stokes Raman spectroscopy in the fingerprint spectral region. / Dudovich, Nirit; Oron, Dan; Silberberg, Yaron.
In: Journal of Chemical Physics, Vol. 118, No. 20, 22.05.2003, p. 9208-9215.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Single-pulse coherent anti-Stokes Raman spectroscopy in the fingerprint spectral region
AU - Dudovich, Nirit
AU - Oron, Dan
AU - Silberberg, Yaron
PY - 2003/5/22
Y1 - 2003/5/22
N2 - Single-pulse vibrational spectroscopy was readily achieved using coherent control techniques. By tailoring the spectral phase of an ultrashort pulse, the interference between quantum processes induced by the various spectral components of the pulse was controlled, leading either to selective population of given Raman levels or to the generation of narrow features in the CARS spectrum by all the populated Raman levels. By applying this principle, high-resolution spectroscopy was demonstrated in the vibrational energy range 700-1400 cm-1. By measuring a complex Raman spectrum of a molecule in this spectral region, the method was found to be robust and practical.
AB - Single-pulse vibrational spectroscopy was readily achieved using coherent control techniques. By tailoring the spectral phase of an ultrashort pulse, the interference between quantum processes induced by the various spectral components of the pulse was controlled, leading either to selective population of given Raman levels or to the generation of narrow features in the CARS spectrum by all the populated Raman levels. By applying this principle, high-resolution spectroscopy was demonstrated in the vibrational energy range 700-1400 cm-1. By measuring a complex Raman spectrum of a molecule in this spectral region, the method was found to be robust and practical.
UR - http://www.scopus.com/inward/record.url?scp=0038549044&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=0038549044&partnerID=8YFLogxK
U2 - 10.1063/1.1568072
DO - 10.1063/1.1568072
M3 - Article
VL - 118
SP - 9208
EP - 9215
JO - Journal of Chemical Physics
JF - Journal of Chemical Physics
SN - 0021-9606
IS - 20
ER -