Abstract
A method for nonlinear spectroscopy with broad-band pulses was presented. This method utilizes strong nonresonant background accompanying all nonlinear processes as a controllable local oscillator. The experimental results showed that by measuring the spectrum of the coherent anti-Stokes Raman signal, it is possible to infer the vibrational energy levels in a band spanning an entire octave.
Original language | English |
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Pages (from-to) | 2730011-2730014 |
Number of pages | 4 |
Journal | Physical Review Letters |
Volume | 89 |
Issue number | 27 |
Publication status | Published - Dec 30 2002 |
ASJC Scopus subject areas
- Physics and Astronomy(all)