TY - JOUR
T1 - Ultrafast Coherent Terahertz Spectroscopy in High Magnetic Fields and Directed Energy Flows in Quantum Dot Assemblies
AU - Crooker, S. A.
AU - Barrick, T.
AU - Hollingsworth, J. A.
AU - Klimov, V. I.
N1 - Copyright:
Copyright 2017 Elsevier B.V., All rights reserved.
PY - 2003/8
Y1 - 2003/8
N2 - We describe the design, construction, and use of fiber-coupled terahertz antennas for performing ultrafast coherent THz spectroscopy directly in the cryogenic bore of high-field magnets. With an aim towards measuring the high-frequency (100 GHz to 2000 GHz) complex conductivity of correlated electron materials in the regime of low temperatures and high magnetic fields, these miniature THz emitters and receivers are demonstrated to work down to 1.5 K and up to 18 T, for eventual use in higher-field magnets. Results from a variety of semiconducting and superconducting samples are presented. This paper also describes a separate effort towards achieving coupling between colloidal semiconductor nanocrystal quantum dots, wherein we realize and study inter-dot communication via resonant (Förster) energy transfer. We present studies of the dynamics of resonant energy transfer in monodisperse and energy gradient (layered) assemblies of CdSe nanocrystal quantum dots. Time- and spectrally-resolved photoluminescence data directly reveal the energy-dependent transfer rate of excitons from smaller to larger dots. Results from layered nanocrystal quantum dot assemblies demonstrate unidirectional energy flows, a first step towards artificial light-harvesting structures. Lastly, time-resolved studies at millikelvin temperatures elucidate the nature of ground-state "dark" excitons in these quantum dots.
AB - We describe the design, construction, and use of fiber-coupled terahertz antennas for performing ultrafast coherent THz spectroscopy directly in the cryogenic bore of high-field magnets. With an aim towards measuring the high-frequency (100 GHz to 2000 GHz) complex conductivity of correlated electron materials in the regime of low temperatures and high magnetic fields, these miniature THz emitters and receivers are demonstrated to work down to 1.5 K and up to 18 T, for eventual use in higher-field magnets. Results from a variety of semiconducting and superconducting samples are presented. This paper also describes a separate effort towards achieving coupling between colloidal semiconductor nanocrystal quantum dots, wherein we realize and study inter-dot communication via resonant (Förster) energy transfer. We present studies of the dynamics of resonant energy transfer in monodisperse and energy gradient (layered) assemblies of CdSe nanocrystal quantum dots. Time- and spectrally-resolved photoluminescence data directly reveal the energy-dependent transfer rate of excitons from smaller to larger dots. Results from layered nanocrystal quantum dot assemblies demonstrate unidirectional energy flows, a first step towards artificial light-harvesting structures. Lastly, time-resolved studies at millikelvin temperatures elucidate the nature of ground-state "dark" excitons in these quantum dots.
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U2 - 10.12693/APhysPolA.104.113
DO - 10.12693/APhysPolA.104.113
M3 - Conference article
AN - SCOPUS:0242353817
VL - 104
SP - 113
EP - 122
JO - Acta Physica Polonica A
JF - Acta Physica Polonica A
SN - 0587-4246
IS - 2
T2 - Proceedings of the 32nd International School of Semiconducting Compounds
Y2 - 30 May 2003 through 6 June 2003
ER -